Can't change album art

in iPod + iTunes + AppleTV edited January 2014
I've been putting a bunch of movies into iTunes recently, and normally they are in mp4 format, but I have a few in .mov. Everything works fine, except that I can't put in album art when it's in the .mov format. It's just set at the first frame of the video, and appears to be unchangeable from within iTunes. Normally I select get info from within iTunes, go to art, delete what's there (it seems to select the first frame of the video by default), and paste in what I want. That doesn't work with the .mov files - it won't let me delete, and I can't figure anything else out.

Any help?
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