3rd Gen iPod Issues with Pictures

in iPod + iTunes + AppleTV edited January 2014
I have a 3rd Gen iPod Nano and add about 200 photos to it using a microsoft and I saved all the photos to My Pictures in specific folders. I took new pictures and I wanted to put them on my iPod, but I could not find the folders with the pictures in them. I checked on iTunes and they said that my iPod was not synced with any folders, but I could see the former pictures on my iPod. I was wondering if there was a way to retrieve those former pictures so I could put them back in the My Pictures folder. Thanks in advance.
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